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After that, Queiroz was appointed senior national team coach in 1991. He had a record of 14 wins in 31 matches. Afterwards, he went on to manage the Portuguese Primeira Divisão team Sporting CP in 1994.He subsequently coached the NY/NJ MetroStars in the United States and the Japanese team, Nagoya Grampus Eight. In between, he found time to author the Q-Report, detailing plans to professionalize the development of footballers in the United States. Queiroz returned to coaching national teams in 1999, when he took the job as head coach of the United Arab Emirates, before becoming head coach of South Africa in 2000.
