Later, he was appointed as the coach of the Persian national team and managed to lead the Persian national team to the championship position in the Asian Nations Cup, defeating the Kuwait national football team in the final of this competition in 1354. The time for the next success of the immigrants came very soon. For the first time in the history of Persian football, the Iranian national football team reached the quarterfinal stage of the 1976 Montreal Olympics under his coaching. Two years later, Mohajerani achieved the greatest honor for himself and Persian football.